Seidel Lab

Helmholtz Center Berlin

Berlin (DE3) · Germany

ERC-funded
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ERC Consolidator Grant · 2023

PHOTO-INDUCED ELECTRON DYNAMICS AT THE TRANSITION-METAL OXIDE–WATER INTERFACE FROM TIME-RESOLVED LIQUID-JET PHOTOEMISSION

Photocatalytic water splitting using transition metal oxides (TMOs) has the potential to play a key role in the sustainable large-scale production of hydrogen. Due to their activity, cost-effectiveness, and stability TMOs are viewed as attractive materials to catalyze water splitting by harnessing solar energy. A major challenge is effectively preventing the recombination of electrons and holes in the TMOs produced upon (solar) light absorption. While these charge recombination processes occur on the pico-to-nanosecond timescale, the whole water splitting process is almost 12 orders of magnitude slower! This huge difference urgently demands a better understand of the underlying mechanisms…

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